The Complete Picture: The Very Best of Deborah Harry and Blondie was a compilation album released on Chrysalis Records in 1991. It contained all of Blondie's biggest hits such as "Heart of Glass", "Sunday Girl", "The Tide Is High", "Atomic" and "Call Me" as well as some of Deborah Harry's solo hits, including the UK Top 10 single "French Kissing In the USA".

The Complete Picture sold well in the UK and reached Number 3. It reached gold status and remained on the charts for 25 weeks. It was released as a double album, containing 5 tracks on each side. However, for the compact disc format, all 20 tracks were released on one CD. A video collection was also released, containing the promotional videos for Koo Koo tracks "Backfired" and "Now I Know You Know" - although these were not included on the album.

Track listing

1. "Heart of Glass" (Faded The Best of Blondie Version) (Harry, Stein) - 3:58
• Performed by: Blondie
2. "I Want That Man" (Bailey, Currie) - 3:41
• Performed by: Deborah Harry
3. "Call Me" (Harry, Moroder) - 3:28
• Performed by: Blondie
4. "Sunday Girl" (Stein) - 3:02
• Performed by: Blondie
5. "French Kissin' in the USA" (Album Version) (Lorre) - 5:10
• Performed by: Debbie Harry
6. "Denis" (Levenson) - 2:18
• Performed by: Blondie
7. "Rapture" (The Best of Blondie Version) (Harry, Stein) - 5:33
• Performed by: Blondie
8. "Brite Side" (Harry, Stein) - 4:34
• Performed by: Deborah Harry
9. "(I'm Always Touched by Your) Presence, Dear" (Valentine) - 2:41
• Performed by: Blondie
10. "Well Did You Evah!" (Porter) - 3:27
• Performed by: Deborah Harry & Iggy Pop
11. "The Tide Is High" (Album Version) (Barrett, Evans, Holt) - 4:35
• Performed by: Blondie
12. "In Love with Love" (Album Version) (Harry, Stein) - 4:30
• Performed by: Debbie Harry
13. "Hanging on the Telephone" (Lee) - 2:22
• Performed by: Blondie
14. "Island of Lost Souls" (7" Edit) (Harry, Stein) - 3:49
• Performed by: Blondie
15. "Picture This" (Destri, Harry, Stein) - 2:56
• Performed by: Blondie
16. "Dreaming" (Harry, Stein) - 3:03
• Performed by: Blondie
17. "Sweet and Low" (Phil Harding Single Mix) (C., Harry) - 4:18
• Performed by: Debbie Harry
18. "Union City Blue" (Harrison, Harry) - 3:20
• Performed by: Blondie
19. "Atomic" (Album Version) (Destri, Harry) - 4:38
• Performed by: Blondie
20. "Rip Her to Shreds" (Harry, Stein) - 3:19
• Performed by: Blondie