Carbon/Silicon recorded four demo CDs: Sample This, Peace; Dope Factory Boogie; The Grand Delusion and The Homecoming. The band's first officially released album, A.T.O.M (A Twist of Modern) debuted on the band's website on 28 July 2006. The next album Western Front followed soon after on October 14, 2006 and included re-recorded versions of their earlier songs. The group's third album, The Crackup Suite was released in March 2007 and is now available for download on their website. The same month it was announced that Leo "Eazykill" Williams, former bandmate of Jones with BAD would play bass for the group, and that Dominic Greensmith formerly of Reef would take up the drum slot. The band further released two EP's plus another album The Last Post and toured, including the Isle of Wight Festival and dates in the USA.
In January 2008, in what is seen as a return their roots, the band played 7 weekly concerts at a tiny venue Inn on the Green in Ladbroke Grove, London. At the first gig, Topper Headon got up and played with the band for two songs. At the final gig, Carbon Casino 7, the Alabama Three took to the stage with Mick and Tony to perform the theme from US TV series, The Sopranos.. Throughout the run, support was provided by West London bands Taurus Trakker, The Rotten Hill Gang,and The Self, songwriter John Byrne, icons Pete Wylie, Glen Matlock, James Dean-Bradfield, John Cooper-Clarke, and new young bands including West London's Dirty Curtains, North London band The Usual Suspects and the Savage Nomads.